NUCLEAR SCIENCE AND ENGINEERING: 90, 374-380 (1985)
Abstract - A personal history of the development of molten salt reactors in the United States is presented. The initial goal was an aircraft propulsion reactor, and a molten fluoride-fueled Aircraft Reactor Experiment was operated at Oak Ridge National Laboratory in 1954. In 1956, the objective shifted to civilian nuclear power, and reactor concepts were developed using a circulating UF4- ThF4 fuel, graphite moderator, and Hastelloy N pressure boundary. The program culminated in the successful operation of the Molten Salt Reactor Experiment in 1965 to 1969. By then the Atomic Energy Commission's goals had shifted to breeder development; the molten salt program supported on-site reprocessing development and study of various reactor arrangements that had potential to breed. Some commercial and foreign interest contributed to the program which, however, was terminated by the government in 1976. The current status of the technology and prospects for revived interest are summarized.
Resumé - Le mémoire traite de l'histoire du développement de réacteurs sels fondus aux Etats Unis du point de vue de l'experience personnelle de l'auteur. Le but initial fut un reaaeur de propulsions d'avion, et une expe'rience denommee Aircraft Reactor Experiment fut entreprise dans l'Oak Ridge National Laboratory en 1954 avec le fluorure fondu corn me combustible. En 1956 le but original fut abandonné en faveur de Ia puissance nucléaire civile, et des conceptions de reacteur furent mises au point basees sur le combustible UF4-ThF circulant, le graphite comme modérateur et Hastelloy N cornme enceinte sous pression. Le programme atteignit son point culminant avec le succes caracterisant l'experience Molten Salt Reactor Experiment poursuivie de 1965 jusqu'á 1969. Les buts vises par l'Atomic Energy Commission s'e'taient ensuite orientes vers le développement du surgenerateur rapide et le programme de reacteurs a sels fondus fut con tin ue' pour appuyer le retraitement sur le terrain de Ia station nucléaire ainsi que l'e'tude de diffe'rentes configurations en pile offrant un potentiel de surrége'ne'ration. 11 y avait un certain nombre de partenaires industrieis et etrangers contribuant au programme qui, cependent, fut arrete' par le gouvernement en 1976. Le me'moire donne un aper de l'état actuel de Ia technologie ainsi que des perspectives pour un renouvellement de l'inte'ret.
Zusammenfassung - Die Geschichte der Entwicklung des Salzschmelzenreaktors in den Vereinigten Staaten wird aus der persönlichen Sicht des Verfassers dargestellt. Ursprüngliches Ziel war ein Antriebsreaktor für Flugzeuge, und im Jahre 1954 wurde im Oak Ridge National Laboratory ein Aircraft Reactor Experiment mit einer Fluoridschmelze als Brennstoff durchgeführt. Im Jahre 1956 änderte sich die Zielrichtung zugunsten des zivilen Sektors der Kernenergie, und es wurden Konzepte für Reaktoren mit umlaufendem UF4-Th4F-Brennstoff, Graphitmoderator und Hastelloy-N-Druck einschluß entwickelt. Das Programm gipfelte in der erfolgreichen Durchführung des Molten Salt Reactor Experiment in den Jahren 1965 bis 1969. Zu diesem Zeitpunkt hatte sich die Atomic Energy Commission für die Brüterentwicklung entschieden, und das Kernschmelzenprogramm wurde ein Unterstützungsprogramm bei der Entwicklung der Wiederaufarbeitung auf Kraftwerksgeländen und bei der Untersuchung verschiedener Reaktoranordnungen, die für den Brutvorgang in Frage kamen. Das Programm fand die Unterstützung einiger interessierter Industriefirmen und ausländischer Partner, wurde aber 1976 von der Regierung eingestellt. Der derzeitige Stand der Technik und Aussichten auf ein Wiederaufleben des Interesses werden im vorliegenden Bericht zusammenfassend dargestellt.
This story of the development of the molten salt reactor (MSR) is
told the way I remember it. For me, it started in 1956 after I had
decided that I would like to become more directly involved in the
development of nuclear power. To do this I needed a new job, and to
get such a job I needed a few references. Thus I wrote to Alvin
Weinberg to see whether he would put in a good word for me.
My acquaintance with Alvin started in 1946-1947 when I was a
student at Oak Ridge's "Clinch College of Nuclear Knowledge," as the
training school under Eugene Wigner and Fred Seitz came to be called.
Alvin, who was then assistant director of the Physics Division, was
one of my teachers and I was tremendously impressed with him. I went
back to a Union Carbide research laboratory in Cleveland, Ohio, at
the end of my year at Oak Ridge, and in late 1947, when It was
decided that Union Carbide was to take over the operation of Oak
Ridge National Laboratory (ORNL), I was called to New York to brief a
few vice-presidents as to who the good guys and the bad guys were.
All I could think to tell them was to get on the good side of Alvin
Weinberg. I told them that he was the natural leader of the place and
that their success would depend on him. I have never told Alvin of
this incident, and I am sure my advice was not necessary for the
Union Carbide officials to recognize Alvin's worth.
When I wrote Alvin for a reference, he responded by asking me to
come to Oak Ridge to head up a program to investigate power reactors
fueled with molten salts. Although I did not know much about molten
salts at the time, the job sounded exciting and I gladly
Molten salt reactors were first proposed by Ed Bettis and Ray
Briant of ORNL during the post-World War II attempt to design a
nuclear-powered aircraft. The attraction of molten fluoride salts for
that program was the great stability of the salts, both to high
temperatures and to radiation. An active development program aimed at
such an aircraft reactor was carried out from about 1950 to 1956. The
Aircraft Reactor Experiment, a small reactor using a circulating
molten fuel salt, operated for several days in 1943 [sic 1953] and
reached a peak temperature of 1620° F. In 1956 interest in the
airplane began to fall off, and Alvin Weinberg wished to see whether
the molten fluoride fuel technology that had been developed for the
aircraft could be adapted to civilian power reactors. Part of his
interest stemmed from the fact that all of the other materials and
coolants being suggested for reactors had been anticipated by the
reactor design group at the Metallurgical Lab oratory in Chicago
during World War II. This was new.
In starting the new civilian program, we had a tremendous head
start from the capable staff and the research under way for the
aircraft program. Our civilian program was in reality a continuation
of the old military program with a few changes in emphasis.
It is my impression that the Division of Reactor Development (DRD)
of the U.S. Atomic Energy Com mission (AEC) never showed much
enthusiasm for the Molten Salt Reactor Program. At the start, in
1956, Alvin had to use all his powers of persuasion with Kenneth
Davis, who was then director of the DRD, to provide us with an
initial $2 million per year to start the program. A couple of years
later the DRD realized that they were supporting too many fledgling
reactor concepts. While each concept could be researched at the
exploratory level with only modest funding, to carry the development
of any concept to fruition would require tremendously larger
expenditures. With funds limited, only a few reactor concepts could
One of the methods employed by the AEC to eliminate reactor concepts was to establish task forces of outside experts to evaluate the reactor concepts and, especially, to point out their weaknesses. After a couple of other reactor concepts had been eliminated by this process, the AEC formed the Fluid Fuels Reactor Task Force to evaluate and compare three different fluid fuel reactors: the aqueous homogeneous, the liquid bismuth, and the MSRs. The task force met In Washington for about two months early in 1959. I was there to represent the molten salt system, Beecher Briggs of ORNL represented the aqueous homogeneous, and Frank Miles from Brookhaven National Laboratory represented the bismuth-graphite reactor. Task force members came from other AEC laboratories, from electric utilities, from architect engineering firms, and from the AEC itself. The first sentence of the Summary of the Task Force Report (TID-8505) was, The Molten Salt Reactor has the highest prob ability of achieving technical feasibility." 1
This conclusion arose from the fact that the molten fluoride salts (a) have a wide range of solubility of uranium and thorium, (b) are stable thermodynamically and do not undergo radiolytic decomposition, (c) have a very low vapor pressure at operating temperatures, and (d) do not attack the nickel-based alloy used in the circulating salt system.
As a result of the task force deliberations, the other two concepts were abandoned and the molten salt system continued its precarious existence. The reactor considered by the Task Force was a converter reactor, not a breeder, and was described as follows:
The reference design molten salt reactor is an INOR-8 (now called Hastelloy N) vessel containing a graphite assembly 12.25 feet in diameter by 12.25 feet high, through which molten salt flows in vertical channels. The fuel salt is a solution composed of 0.3 mole percent UF4 13 mole per cent ThF4, 16 mole percent BeF2, and 70.7 mole percent 7LiF. The fuel salt is heated from 1075° F to 1225° F in the core and is circulated from the reactor vessel to four primary heat exchangers by four fuel pumps. A barren coolant salt is used as the intermediate heat exchange fluid.1
It is interesting to me that this reactor description prepared hurriedly in early 1959 differs only in minor detail from the MSR designs of the 1970s.
Until late 1959 our exploration of MSRs was not focused sharply on the breeding possibilities of the system, although we always preferred high conversion ratio designs in our studies. Starting in 1960, however, the financial support of the Molten Salt Reactor Program was dependent on its breeding possibilities, and thereafter the program was focused on the molten salt breeder reactor (MSBR). Thermal breeders have only a small breeding margin, and, to breed comfortably, fission products must be kept at low concentrations. This means that the fuel must be purified frequently. The fact that the molten salt fuel is a liquid helps in this respect, since the gaseous fission products come off continuously and the fuel can be purified from other fission products by suitable liquid extraction methods. In principle, this purification is much easier for MSRs than it is for solid fuel reactors, since the steps of dissolution and refabrication of the fuel are avoided.
Over the course of years, suitable processing methods were found
so that the single fluid reactor described above could become a
breeder. In 1960, however, our limited knowledge of processing
chemistry forced us to consider breeder reactors in which the fuel
(fissile uranium) was kept in one fluid and the fertile material
(thorium) was in a separate fluid. Both fluids circulated through the
reactor, but were kept separate by walls of graphite.
By the end of 1959, our engineering development program had
proceeded far enough that we felt justified in proposing an MSR
experiment (MSRE), but getting money and permission appeared
difficult. Then one day I heard a rumor that Frank Pittman, who had
succeeded Ken Davis as director of the DRD, had expressed interest in
funding as many as four "quick and dirty" reactor experiments
provided that each one should cost less than a million dollars. As I
remember it, I wrote a proposal that night and submitted it through
channels the next day. I outlined the general features of the
reactor, and by analogy with another reactor system for which a cost
estimate had been made. I came up with a cost estimate of $4.18
million. The proposal was accepted, although by the time the design
had been detailed the cost estimate had doubled.
The conceptual design of the MSRE was arrived at as follows. To
keep the reactor simple we intended to simulate only the fuel stream
of a two-fluid breeder reactor, so that no thorium fluoride was
included. We wanted the neutron spectrum to be near thermal, as it
would be in a commercial reactor, and since graphite was the
moderator, this dictated the minimum physical size. The moderator was
in the form of a 1.37-m-diam x 1.62-m-high right circular cylinder.
Had it been smaller, the neutron leakage would have caused the
neutron spectrum to be more energetic than we wished. We would have
liked to have a higher power density, but cost considerations limited
us to ~10 MW of heat. There was also another reason for limiting the
power of the reactor. The AEC accounting rules at the time allowed us
to build a 10-MW reactor as an experiment, using operating funds. A
higher power reactor would have required us to obtain a capital
appropriation and would have limited our freedom to make changes.
Actually we miscalculated the heat transfer characteristics and the
reactor operated at only 8 MW.
I ceased being director of the MSR program in 1960, at which time
capable engineers took over for the construction of the MSRE and the
later development work. However, I maintained my strong interest in
the program during my tenure as deputy director of ORNL and even
after leaving in 1970.
Design of the MSRE started in the summer of 1960 and construction
started 18 months later, at the beginning of 1962. The reactor went
critical in June 1965, and was briefly at full power a year later.
After a shakedown period, reliable operation was achieved in December
1966, when a 30-day continuous run was made at full power. While
carrying out numerous experiments, the reactor was operated at full
power most of the time during the next 15 months, after which the
235U was removed from the fuel salt and later replaced with 233U. The
reactor was operated with 233U as the fuel from January through May
1969. This was the first time 233U had been used as a reactor fuel,
and AEC Chairman Glen Seaborg and Ray Stoughton, codiscoverers of
233U, were present when the reactor first went critical with 233U
During the remainder of 1969, the reactor was devoted to a number
of experiments, including xenon stripping, fission product
deposition, tritium behavior, and plutonium additions. Operation was
finally terminated in December 1969 so that the available funds could
be applied to other development areas.
In 1962 the AEC first took a position strongly favoring the
development of breeder reactors. This position was spelled out in its
1962 "Report to the President." In that report two breeder reactors
were described and discussed. One was the familiar
liquid-metal-cooled fast breeder reactor (LMFBR) using the 238U-Pu
breeding cycle, and the other was the molten salt fueled thermal
breeder using the 233U-Th cycle. Somewhat surprisingly, the report
devoted about 60% as much favorable space to the molten salt thermal
breeder as to the fast breeder, despite the much broader countrywide
participation in the fast breeder program.
The AEC's 1962 "Report to the President" was written while the
MSRE was under construction, but apparently we had proceeded far
enough with our development program to impress the Subcommittee on
Reactors of the General Advisory Committee with the value of the
molten salt system. As soon as the "Report to the President"
presented its justification for the development of breeder reactors,
however, the existent Liquid Metal Cooled Reactors Department of the
DRD proposed an elaborate and wide-ranging program for the
development of the LMFBR concept, and that program began to gain
momentum. On the other hand, those of us involved in the MSR program
chose to wait until the MSRE had operated success fully before trying
to expand our program. This, we thought, was the prudent thing to do,
but by the time we were prepared to go for a larger reactor, the
momentum and money needs of the LMFBR program were massive and there
was no interest in funding a competitor.
The MSRE was a very successful experiment, in that it answered
many questions and posed but a few new ones. Perhaps the most
important result was the conclusion that it was quite a practical
reactor. It ran for long periods of time, and when maintenance was
required, it was accomplished safely and without excessive delay.
Also, it demonstrated the expected flexibility and ease of handling
the fuel. As mentioned above, it was the first reactor in the world
to operate with 233U as the sole fuel, and the highly radioactive
233U used would have been extremely difficult to handle if it had had
to be incorporated into solid fuel elements. In preparation for the
run with 233U, the 235U was removed from the carrier salt in 4 days
by the fluoride volatility process. This process decontaminated the
218 kg of uranium of gamma radiation by a factor of 4 x
109 so that it could be handled with out shielding. As an
aside, this equipment used for the MSRE was sufficiently large so
that it could satisfactorily handle all of the fuel processing needs
for a 1000-MW molten salt converter reactor (MSCR), about which I
will say more later.
Three problems requiring further development turned up during the
construction and operation of the MSRE. The first was that the
Hastelloy N used for the MSRE was subject to a kind of "radiation
hardening," due to accumulation of helium at grain boundaries. Later,
it was found that modified alloys that had fine carbide precipitates
within the grains would hold the helium and restrain this migration
to the grain boundaries. Nevertheless, it is still desirable to
design well-blanketed reactors in which the exposure of the reactor
vessel wall to fast neutron radiation is limited.
The second problem concerned the tritium produced by neutron
reactions with lithium. At high temperatures the radioactive tritium,
which is, of course, chemically like hydrogen, penetrates metals
quite readily, and unless captured in some way, would appear in the
steam generators and reach the atmosphere. After considerable
development work, it was found that the intermediate salt coolant, a
mixture of sodium fluoride and sodium fluoroborate, would capture the
tritium and that it could be removed and isolated in the gas purge
The third problem came from the discovery of tiny cracks on the
inside surface of the Hastelloy N piping for the MSRE. It was found
that these cracks were caused by the fission product tellurium. Later
work showed that this tellurium attack could be controlled by keeping
the fuel on the reducing side. This is done by adjustment of the
chemistry so that about 2% of the uranium is in the form of
UF3, as opposed to UF4. This can be controlled
rather easily now that good analytical methods have been developed.
If the UF3 to UF4 ratio drops too low, it can
be raised by the addition of some beryllium metal, which, as it
dissolves, will rob some of the fluoride ions from the uranium.
As solutions to these new problems became available, those of us
familiar with the technology believed that we were ready for the next
step, the construction of a reactor producing modest amounts of
electrical power, or at least the development of the equipment needed
for such a reactor. In any case, productive continuation of the MSR
program in the United States would soon require funds an order of
magnitude greater than previous expenditures.
In 1972 ORNL proposed a major development program that would
culminate in the construction and operation of a demonstration
reactor called the Molten Salt Breeder Experiment. The program was
estimated to cost a total of $350 million over a period of 11 yr.
However, those who would have had to approve such a program were
already heavily committed to the LMFBR and guiding a very expensive
development program that would be spending about $400 million each
year by 1975. It was asking too much of human nature to expect them
to believe that a much less expensive program could be effective in
developing a competing system, and the ORNL proposal was rejected. In
January 1973, ORNL was directed to terminate MSR development work.
For reasons I do not understand, the program was reinstated a year
later, and in 1974 ORNL submitted a more elaborate proposal with
suitably inflated costs calling for about $720 million to be spent
over an 11-yr period. This last proposal was also rejected, and in
1976 ORNL was again ordered to shut down the MSR program "for
The decision to cut off the funding for the MSR program was
supported by an "evaluation" of the MSBR (1972) prepared internally
by the Division of Reactor Development and Technology in response to
a request from the Office of Science and Technology. Although this
report contained no overt recommendations, the Conclusions section,
after granting some attractive features of the MSR, emphasized the
difficulty of solving a number of problems, including those described
above. It was stated that after realistic solutions for these
problems had been demonstrated, proceeding toward engineering
development would require "reasonable assurances that large scale
government and industrial resources can be made available on a
continuing basis in light of other commitments to the commercial
nuclear power program and higher priority energy developments." This
was, of course, true.
This evaluation was prepared before the solutions to the tritium
evolution and tellurium cracking problems were known. On a recent
trip to Japan, I was asked the following question by a group of
engineers who were thoroughly familiar with MSR technology:
"Concerning the MSBR development program, the U.S. AEC pointed out
the following major technological problems in 1972, namely the
problem on the materials, the tritium and fuel salt chemical
processing. And we think that most of the above problems have been
settled by the splendid effort of R&D; performed by ORNL
thereafter, but how was it evaluated in the U.S.?" I do not believe
that such an evaluation was made or that the Department of Energy is
prepared to make one.
For the several groups of enthusiasts for molten salt technology in other countries, the reasons for the demise of the U.S. program are important. It is difficult for them to overcome the stigma of abandonment of the MSR by the country of its origin. In my opinion, these are the major factors contributing to the cessation of the program.
1. The political and technical support for the program in the United States was too thin geographically. Within the United States, only in Oak Ridge, Tennessee, was the technology really understood and appreciated.
2. The MSR program was in competition with the fast breeder program, which got an early start and had copious government development funds being spent in many parts of the United States. When the MSR development program had progressed far enough to justify a greatly expanded program leading to commercial development, the AEC could not justify the diversion of substantial funds from the LMFBR to a competing program.
It was often suggested by the DRD that evidence of industrial
support for the MSR was needed to gain AEC enthusiasm. However, the
evidence available for this support was ignored.
At least two privately funded technology evaluation and design
studies of the MSR were made. One was carried out in 1970 by a group
called the Molten Salt Breeder Reactor Associates, headed by Black
and Veach and including five Midwest utilities. The other study was
done by The Molten Salt Group, which was headed by Ebasco Services,
Inc., and included 5 large industrial firms and 15 utilities. Both of
these studies reported favorably on the promise of the system. The
Molten Salt Group concluded in 1971 that the existing technology was
sufficient to justify construction of a molten salt demonstration
About 10 yr have elapsed since the demise of the active MSR
development program at ORNL. In that interval several changes have
occurred that might have some influence on how the MSR is
Foremost has been the decreased rate of expansion of electricity
use in developed countries. This has sharply reduced the expected
rate of building new nuclear power plants by as much as an order of
magnitude. As a result, we no longer expect a crisis in the
availability of uranium for at least 50 yr. Even with some renewed
growth, it is unlikely that breeders will be needed before 2035 to
2050. With this delay in the need for breeders, the primary current
interest should be for reactors that are economical and that have
other features of merit that might encourage a revival of new reactor
construction. Thus, there is no need for the MSR to emerge as a
full-blown breeder, and it should now be considered on its merits as
a relatively simple, low cost, converter reactor, the MSCR. The fact
that the MSCR can be developed into a breeder at the suitable time by
the addition of chemical processing equipment should be regarded as a
positive feature. Full engineering development of the known methods
for accomplishing this, however, can be deferred for decades.
Another major change is the very high capital costs that are
reported in building fast breeder reactors. The result is that the
LMFBR will not be competitive with light water reactors (LWRs) until
natural uranium reaches astronomically high costs; in fact, until it
attains levels it may never reach in the next century. Thus, fast
reactors as currently designed will not be economically competitive
for perhaps two generations (of people). By the time they are
competitive, a whole new crop of nuclear engineers will have to learn
Off hand one might think that the high cost of LMFBRs would open
the door to other advanced reactor systems, such as the MSCR. The
practical effect is negative, however, since the new information
casts doubt on the projected costs of all advanced reactor systems,
and this presumption is difficult to overcome without actual
experience with hardware. In 1970 a careful detailed estimate was
made of the capital cost of an MSR and it turned out to be within 1%
of the cost of an LWR. Construction experience is needed, however, to
verify such a cost estimate.
Like the LMFBR, the MSR has an intermediate heat transfer loop to isolate the steam generators from radioactive fluids. However, there are basic reasons for expecting MSCR capital costs to be lower than those for the LMFBR:
1. The fuel handling system will be much simpler.
2. The molten salts have a much higher heat capacity per unit volume than sodium, so that the physical size of pumps and piping will be smaller.
3. There is no threat of a "core disruptive accident" with the MSCR, so that safety-related equipment can be simpler.
4. The molten salts have a much lower thermal conductivity than sodium, so that sudden coolant temperature changes will provide less thermal shock to system components.
5. The coolant is more compatible with water than is sodium, so that there should be fewer problems in the design and maintenance of steam generators.
On the other hand, it should be remembered that the development of large engineering components for the MSCR is in a primitive state and that any future development program would surely reveal new difficulties of uncertain magnitude. Furthermore, the high degree of radioactivity of the MSCR's primary system will present problems of design for remote maintenance. The continuing development of robots ought to be of some help here.
Another change is the effective moratorium on fuel processing for
LWRs, resulting from fears of plutonium weapons proliferation and
from higher projected costs of plutonium recycling. As a result,
large stockpiles of plutonium will be accumulating, stored mostly in
spent fuel elements. The safe use of this plutonium is one of the
reasons for the current interest in MSRs in Japan. Preliminary
calculations indicate the possibility of obtaining additional energy
out of spent LWR fuel by dissolving it in a fluoride salt and burning
it in an MSCR.
The fear of weapons proliferation has also spurred an interest in
reactors that do not use highly enriched fuels and that avoid fuel
reprocessing. A recent quite sophisticated study at ORNL has shown
how an MSCR using thorium as the fertile material but fueled with 20%
enriched uranium could be operated for 30 yr without any processing
of the fuel. There would be periodic additions of the 20% enriched
uranium, but no need to remove fission products other than those
coming off naturally in the gas purge system. Even under these
extreme conditions, the lifetime average conversion ratio is ~0.80. I
was personally surprised at the favorable result of that study, which
illustrates another way that the MSR technology could be used if
A social change within the last few years is the increased
sensitivity of the public to the possibility of reactor accidents.
The MSRs deserve consideration on this score, especially because
catastrophic accidents appear to be extremely unlikely. Although the
entire primary system of an MSR is highly radioactive, there is
little driving force to make the activity escape. Thus, with proper
design of the containment, the public should be well protected.
For the foreseeable future, any newly proposed reactor must
compete with the LWR. Because the MSCR's fuel cycle cost will be
lower, it is possible that it can compete with the LWR on a cost
basis. I believe the two most important considerations favoring the
MSR, however, are its versatility in being able to use any fuel and
its ability to be ultimately transformed into a breeder, thus solving
the electric power problem for millennia.
What of the future? The details of the technology developed for the MSR at Oak Ridge are exceedingly well documented, and the knowledge, as preserved on paper, is available to any group wishing to pursue a new development effort.2-8 There continues to be a significant amount of international interest in molten salts.9-15 Sophisticated research on the chemistry and technology is going on at several Japanese universities and there is some industrial interest there. A new engineering development project has been started in Italy for which I have great hopes. Certain individuals in France, India, the USSR, and other countries are strongly interested. It is possible that one of these centers of interest will persevere and ultimately achieve commercial success. Mr. Weinberg and I would be overjoyed.
1 H. G. MacPHERSON et al., "Summary Report, Fluid Fuels Reactor Task Force," TID-8505, U.S. Atomic Energy Commission (I 959).
2. R. C. BRIANT and A. M. WEINBERG, NucI.Sci. Eng., 2, 797 (1957).
3. J. R. ENGEL, H. F. BAUMAN, J. F. DEARING, W. R. GRIMES, E. H. McCOY, and W. A. RHOADES, "Conceptual Design Characteristics of a Denatured Molten-Salt Reactor with Once-Through Fueling," ORNL/TM-7207, Oak Ridge National Laboratory (1980).
4. "Molten-Salt Reactor Program Semi-Annual Progress Report for Period Ending February 29, 1976," ORNL-5132, Oak Ridge National Laboratory (1976). This is the last of the 36 periodic ORNL Program Reports.
5. M. W. ROSENTHAL, P. N. HALBENREICH, and R. B. BRIGGS. "The Development Status of Molten-Salt Breeder Reactors," ORNL-4812, Oak Ridge National Laboratory (1972). 6. H. G. MacPHERSON, React. Technol., 15, 136 (1972).
7. A. M. PERRY and A. M. WEINBERG, Annual Review of Nuclear Science, 22, 317 (1972).
8. "A Review of Molten-Salt Reactor Technology," NucI. AppI. Technol., 8, 2 (1970). This issue is a compilation of eight articles by 27 authors from Oak Ridge National Laboratory summarizing the history and technology of MSRs through 1969.
9. K. FURUKAWA et al., "Accelerator Molten-Salt Breeding System," Proc. 1st Int. Symp. Molten Salt Chemistry and Technology, p. 399. Kyoto (1983).
10. R. ISHIGURO et al., "Research on Molten Salt Reactors,' Research on Thorium Fuel, Chap. VI, SPEY 9, Ministry of Education, Science, and Culture, Tokyo (1984).
11. V. M. NOVIKOV, "Molten Salt Advanced and Emerging Nuclear Systems: Flexible Energy Option," 3rd Int. Conf. Emerging Nuclear Energy Systems, Helsinki (June 1983).
12. M. TAUBE, Atomkernenergie, 7, 7 (1981).
13. D. D. SOOD, "Molten Salt Reactor Concept," Board of Research in Nuclear Science, Bombay (1980).
14. M. HERY, A. LECOCQ, and F. FAUGERAS, "Results of and Prospects for Studies on Molten Salt Nuclear Reactors," Proc. 1st Int. Symp. Molten Salt Chemistry and Technology, p. 423, Kyoto (1983).
15. L. F. C. REICHLE, "MSR (Pu Converters) and MSBRs in Commercial Nuclear Power Systems," Proc. 1977 Salzburg Conf. Nuclear Power and Its Fuel Cycle, 1, 531, International Atomic Energy Agency, Vienna (1977).